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It happened shortly after 3 p.m. at the SECU location at 4262 Louisburg Road.
No one was injured.
According to surveillance footage, the man displayed a handgun.
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Police originally reported two men were responsible for the crime; however, they said one of the accused was actually a witness.
The case remains under investigation.
Anyone with information that might assist the investigation of the incident is asked to call Raleigh CrimeStoppers at (919) 834-HELP or visit raleighcrimestoppers.org for text and email reporting options. CrimeStoppers pays cash rewards for anonymous tips that help solve cases.