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Allana N. Mozelle, 32, of the 500 block of Melody Lane in Cameron, died Thursday, the sheriff's office said.
Her husband, Teamus Maurice Mozelle, 35, of the same address, was arrested Friday in New Bern.
He has been charged with one count of murder and one count of possession of a firearm by a convicted felon.
New Bern police officers assisted in finding Mozelle and taking him into custody.
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He'll be returned to Harnett County for processing.
On Sunday, police responded to a call of an accidental shooting at the Mozelle residence. Allana Mozelle was taken by Spout Springs EMS to Cape Fear Valley Hospital. She was later transferred to UNC Hospital in critical condition.