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Authorities arrested 23-year-old Jacob Gardea of Albuquerque, New Mexico, just hours after FBI agents joined the investigation.
Officials said he is accused of kidnapping 13-year-old Aubrey Joelle Acree.
Police said an eyewitness saw Aubrey getting into a vehicle with him near Harris Henrietta Road in Mooresboro on Sunday night.
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Gardea is facing child abduction charges in North Carolina.
Video is from a previous version of this story.