Jones, 36, is now charged with attempted first-degree murder in the shooting of Trooper Daniel Harrell; previously, he was charged with assault with a deadly weapon with intent to kill inflicting serious injuries and assault on a law enforcement officer.
Two other suspects, 40-year-old William Boswell and 25-year-old Bryan Mullins, were arrested in the incident.
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Both were charged with possession of a stolen motor vehicle.
A girlfriend of the two said they were in the wrong place at the wrong time.
'Nothing to do with it:' Girlfriend of suspect in shooting of trooper said he's innocent
Harrell, who was shot in the neck, was released from the hospital on Wednesday.
On Tuesday, a judge set Jones' bond at $1.02 million.
He is due back in court on Friday.